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Endogenous stimuli strategies make use of biochemical differences within the TME, including extracellular and intracellular pH gradients, altered redox status, overexpression of proteases and hypoxic conditions [46, 47, 49]

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The 1 H NMR spectrum of unknown-1 (Figure S3) showed an unusual aromatic first-order (large chemical shift separations and clear coupling pattern) spin-system AMX, where the aromatic protons at H 6.42 ppm (d, J = 8.1 Hz, 1H) and 6.15 ppm (d, J = 8.0 Hz, 1H) were low-shifted in comparison with those of 7-HMG at H 7.20 ppm (d, J = 7.8 Hz, 1H), and 6.73 ppm (d, J = 7.8 Hz, 1H)

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